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Org. Lett. - Ni(II)/Zn Catalyzed Reductive Coupling of Aryl Halides with Dipheny

2014-4-22 23:56| 发布者: Mcdull| 查看: 2123| 评论: 0|原作者: Metalcarbene|来自: 捷报频传

摘要: Remarks: 和学院赵玉芬老师课题组的合作课题。投Angew被拒改投OL,主要贡献在计算部分,按照其中一个referee的要求已将相关部分移至SI。
Letter
Ni(II)/Zn Catalyzed Reductive Coupling of Aryl Halides with Diphenylphosphine Oxide in Water

Xinghua Zhang†, Huizhi Liu†, Xiaomei Hu†, Guo Tang*†, Jun Zhu*‡, and Yufen Zhao†§
Department of Chemistry and Key Laboratory for Chemical Biology of Fujian Province, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, Fujian, China, Department of Chemistry and Fujian Provincial Key Laboratory of Theoretical and Computational Chemistry, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, Fujian, China, and Key Laboratory of Bioorganic Phosphorus Chemistry and Chemical Biology (Ministry of Education), Department of Chemistry, Tsinghua University, Beijing 100084, China
Org. Lett., Article ASAP
DOI: 10.1021/ol201141m
Publication Date (Web): May 27, 2011
Copyright © 2011 American Chemical Society
t12g21@xmu.edu.cn; jun.zhu@xmu.edu.cn, †

Department of Chemistry and Key Laboratory for Chemical Biology of Fujian Province, College of Chemistry and Chemical Engineering, Xiamen University.
, ‡Department of Chemistry and Fujian Provincial Key Laboratory of Theoretical and Computational Chemistry, College of Chemistry and Chemical Engineering, Xiamen University.
, §Tsinghua University.

Abstract
ol-2011-01141m_0008.gif
P-Arylation in water has been developed via cross-coupling of aryl halides with diphenylphosphine oxide (Ph2P(O)H) and (RP)-(−)-menthyl benzylphosphinate catalyzed by NiCl2·6H2O/Zn under relatively mild conditions.

http://pubs.acs.org/doi/abs/10.1021/ol201141m

Remarks: 和学院赵玉芬老师课题组的合作课题。投Angew被拒改投OL,主要贡献在计算部分,按照其中一个referee的要求已将相关部分移至SI。

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